Large-scale screening of high-entropy materials for superionic solid electrolytes (opens in new tab)

Solid electrolytes have emerged as a promising alternative to conventional liquid electrolytes that have posed safety concerns. However, the relatively low ionic conductivity of solid electrolytes is one of the challenges for their practical application. In this work, we study high-entropy materials over a wide chemical space as a combinatorial strategy to enhance the ionic conductivity of solid electrolytes by up to orders of magnitude. To this end, we developed an iterative search framework...